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[2019]
Formate oxidase (FOx) from Aspergillus oryzae: one catalyst to promote H2O2‐dependent biocatalytic oxidation reactions
Tieves F, Willot SJ-P, van Schie MMCH, Rauch MCR, Younes SHH, Zhang W, Dong J, Gómez de Santos P, Robbins JM, Bommarius B, Alcalde M, Bommarius AS, Hollmann F
Angew. Chem. Int. Ed., 58: 7873-7877, 10.1002/anie.201902380
An increasing number of biocatalytic oxidation reactions rely on H2O2 as clean oxidant. The poor robustness of most enzymes towards H2O2, however, necessitates more efficient [...]
[2019]
Selective synthesis of 4-hydroxyisophorone and 4-ketoisophorone by fungal peroxygenases
Aranda C, Municoy M, Guallar V, Kiebist J, Scheibner K, Ullrich R, del Río JC, Hofrichter M, Martínez AT, Gutiérrez A
Catal. Sci. Technol., 9: 1398-1405
The recently discovered unspecific peroxygenases (UPOs) from the ascomycetes Chaetomium globosum and Humicola insolens were capable of selectively hydroxylating isophorone [...]
[2018]
Description of a Non-Canonical Mn(II)-Oxidation Site in Peroxidases
Fernandez-Fueyo E, Davó-Siguero I, Almendral D, Linde D, Baratto MC, Pogni R, Romero A, Guallar V, Martínez AT
ACS-Catalysis, 8: 8386-8395
A dye-decolorizing peroxidase (DyP) from Pleurotus ostreatus (PosDyP4) catalyzes the oxidation of Mn2+ to Mn3+, in the presence of H2O2, with an efficiency similar to the [...]
[2018]
Selective synthesis of the resveratrol analogue 4,4′-dihydroxy-trans-stilbene and stilbenoids modification by fungal peroxygenases
Aranda C, Ullrich R, Kiebist J, Scheibner K, del Río JC, Hofrichter M, Martínez AT, Gutiérrez A
Catal. Sci. Technol., 8: 2394-2401
This work gives first evidence that the unspecific peroxygenases (UPOs) from the basidiomycetes Agrocybe aegerita (AaeUPO), Coprinopsis cinerea (rCciUPO) and Marasmius rotula [...]
[2018]
Self-sustained enzymatic cascade for the production of 2,5-furandicarboxylic acid from 5-methoxymethylfurfural
Carro J, Fernandez-Fueyo E, Fernández-Alonso C, Cañada J, Ullrich R, Hofrichter M, Alcalde M, Ferreira P, Martínez AT
Biotechnol. Biofuels, 11: 86-96
Background
2,5-Furandicarboxylic acid is a renewable building block for the production of polyfurandicarboxylates, which are biodegradable polyesters expected to substitute [...]